This article presents the study of library Automation problems faced by the library staff & users of Delhi and Uttarakhand based Libraries. For this purpose a well-structured questionnaire was designed to know the opinions, functions, activities, using of E-resources, behavior, reading habits, & other different activities done through the E-resources for the staff/users of libraries of UK & Delhi. The result of the survey provides useful information about the automation, information scene, and application, utilization & awareness of computer-based products & services in the performance of different library operation & function. It has added a new dimension to the library services like E-learning, E-library E-books, E-Journals, E-governance etc. There are many problems for maintenance and application of computer-based services to the users and staff of the library but the most of all users and staff are interesting to use Electronic resources day to day. This paper also reveals on the basis of the result of the survey, some suggestion has been forwarded for the effective use of a different Electronic mode of services and activities in present automated libraries environment in Uttarakhand and Delhi also.